This chip is 35-45 years old(circa 1978?) and from what I've managed to find googling it, only NEC may have the rest of the 259-page datasheet in some dusty file cabinet, while only the first 3-pages seem to be available online. This chip is very complicated and you haven't a chance to even start to get it to work without spending days studying the full datasheet.
Find some video controller chip that is newer, well-documented. It will work better, be easier to use, less expensive, less power-hungry, etc.
Better yet, Google for Nextion simple to interface and very inexpensive displays.
I would say your only chance would be to reverse engineer an early 8080 or Z80 CPM computer video board using this chip.