The '181 has already been done: http://www.righto.com/2017/01/die-photos-and-reverse-engineering.html
Thanks!
That is a really great investigation and report into what is inside a 74181. Their detailed explanation of how the transistors work, to make the overall circuit, is just brilliant!
Anyway, nice find.
If decapping TTL chips. The 74181's would still be the (top) one to go for, on the basis that it is one of the biggest and most complicated (of the "older" TTL chip parts). It has a lot of the functionality of a microprocessor, and yet was released before them and used in many historically important computers, of the time.
I.e. It is so big and functional, that it makes it very interesting.
Simple gates, e.g. 7400 Quad Nand, are still interesting. But the very complicated ones (like the 74181), add a lot to how interesting it is (at least for me).
I'm not sure if the OP is going to only do TTL chips which have not yet been publicly decapped, or if they are doing them all, regardless. I get the impression they (OP) are doing this independently of any other works, available on the internet.